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Influence of gold diffusion doped on phase formation superconducting and microstructure properties ofBi1 8Pb0 35Sr1 9Ca2 1Cu3Oy superconductors      
Yazarlar
Prof. Dr. Özgür ÖZTÜRK
Kastamonu Üniversitesi, Türkiye
Mustafa Akdoğan
Abant İzzet Baysal Üniversitesi, Türkiye
Cabir Terzioğlu
Abant İzzet Baysal Üniversitesi, Türkiye
A Gencer
Özet
We report on low-field magnetic properties of gold diffusion-doped Bi 1.8Pb0.35Sr1.9Ca2.1Cu 3Oy superconducting bulk samples by performing ac susceptibility measurements. The undoped samples were prepared by the standard solid-state reaction method. Doping of Bi1.8Pb0.35Sr 1.9Ca2.1Cu3Oy was carried out by means of Au-diffusion during sintering from an evaporated gold film on pellets. To investigate the effect of gold-diffusion and diffusion-annealing duration on transport, magnetic and microstructure properties of the superconducting samples we performed magnetoresistivity, scanning electron microscopy (SEM) and X-ray diffraction (XRD) measurements. The ac susceptibility as a function of temperature measurements were carried out at different values of the ac magnetic field amplitudes (Hac) in the range between 20A/m and 320 A/m for 211 Hz. The imaginary part of ac susceptibility measurements is used to calculate intergranular critical current density Jc(Tp) using the Bean Model. Jc(Tp) is seen to increase from 60 A cm -2 to 90 A cm-2 with increasing diffusion-annealing time from 10 h to 50 h. The peak temperature, Tp, in the imaginary part of the ac susceptibility is shifted to a lower temperature with decreasing diffusion-annealing duration as well as increasing ac magnetic fields. The force pinning density (αjj (0)) increased with increasing diffusion annealing time. The value of Tc in gold-diffused samples, in comparison with the undoped samples, increased from 100 0.2 K to 104 0.2 K. It was observed that the value of Tc-offset of the gold-doped samples enhanced with further increasing diffusion-annealing duration. XRD patterns and SEM micrographs are used to obtain information about Bi-2223 phase ratio, lattice parameters and grain size of the samples. Gold doping enhanced the formation high-Tc phase and increased the grain size. The possible reasons for the observed improvements in transport, microstructure and magnetic properties due to Au diffusion and diffusion-annealing time were discussed. © 2009 IOP Publishing Ltd.
Anahtar Kelimeler
Makale Türü Özgün Makale
Makale Alt Türü SSCI, AHCI, SCI, SCI-Exp dergilerinde yayımlanan tam makale
Dergi Adı Journal of Physics: Conference Series
Dergi ISSN 1742-6596
Dergi Tarandığı Indeksler SCI
Makale Dili İngilizce
Basım Tarihi 03-2009
Cilt No 153
Sayfalar 12024 /
Doi Numarası 10.1088/1742-6596/153/1/012024
Makale Linki http://stacks.iop.org/1742-6596/153/i=1/a=012024?key=crossref.e912ba478b3dc53cd18ad542f30a380e