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Fast and Highly Sensitive Ionic-Polymer-Gated WS2 -Graphene Photodetectors       
Yazarlar
Jake D. Mehew
Dr. Öğr. Üyesi Selim ÜNAL Dr. Öğr. Üyesi Selim ÜNAL
Türkiye
Elias Torres Alonso
Gareth F. Jones
Saad Fadhil Ramadhan
Monica F. Craciun
Saverio Russo
Özet
The combination of graphene with semiconductor materials in heterostructure photodetectors enables amplified detection of femtowatt light signals using micrometer-scale electronic devices. Presently, long-lived charge traps limit the speed of such detectors, and impractical strategies, e.g., the use of large gate-voltage pulses, have been employed to achieve bandwidths suitable for applications such as video-frame-rate imaging. Here, atomically thin graphene–WS2 heterostructure photodetectors encapsulated in an ionic polymer are reported, which are uniquely able to operate at bandwidths up to 1.5 kHz whilst maintaining internal gain as large as 106. Highly mobile ions and the nanometer-scale Debye length of the ionic polymer are used to screen charge traps and tune the Fermi level of the graphene over an unprecedented range at the interface with WS2. Responsivity R = 106 A W−1 and detectivity D* = 3.8 × 1011 Jones are observed, approaching that of single-photon counters. The combination of both high responsivity and fast response times makes these photodetectors suitable for video-frame-rate imaging applications.
Anahtar Kelimeler
graphene | ionic-polymer gating | photodetectors | van der Waals heterostructures | WS 2
Makale Türü Özgün Makale
Makale Alt Türü SSCI, AHCI, SCI, SCI-Exp dergilerinde yayımlanan tam makale
Dergi Adı Advanced Materials
Dergi ISSN 0935-9648
Dergi Tarandığı Indeksler SCI
Makale Dili İngilizce
Basım Tarihi 04-2017
Cilt No 29
Sayı 23
Doi Numarası 10.1002/adma.201700222
Makale Linki http://dx.doi.org/10.1002/adma.201700222
BM Sürdürülebilir Kalkınma Amaçları
Atıf Sayıları
SCOPUS 111
Google Scholar 131
Fast and Highly Sensitive Ionic-Polymer-Gated WS2 -Graphene Photodetectors

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